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Browsing Department of Chemistry by Title
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(Massachusetts Institute of Technology, 1965)
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(Massachusetts Institute of Technology, 1999)
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(Massachusetts Institute of Technology, 2009)Dinitrogen cleavage by Mo(N[t-Bu]Ar)3 (Ar = 3,5-C6H3Me2) proceeds through the intermediate ([mu]-N2)[Mo(N[t-Bu]Ar)3]2 before forming N=Mo(N[t-Bu]Ar)3 as the product. Both the intermediate bridging N2 complex and the nitride ...
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(Massachusetts Institute of Technology, 2007)Non-heme carboxylate-bridged diiron centers in the hydroxylase components of the bacterial multicomponent monooxygenases activate dioxygen at structurally homologous active sites. Catalysis requires the management of four ...
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(Massachusetts Institute of Technology, 1995)
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(Massachusetts Institute of Technology, 1977)
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(Massachusetts Institute of Technology, 1974)
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(Massachusetts Institute of Technology, 1974)
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(Massachusetts Institute of Technology, 2010)[image] The proposed biogenesis of the ladder polyethers features a dramatic series of epoxide opening reactions, elegantly accounts for the structural and stereochemical features of all related natural products, and, in ...
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(Massachusetts Institute of Technology, 2008)I. Synthesis of Substituted Pyridine Derivatives via the Ruthenium-Catalyzed Cycloisomerization of 3-Azadienynes. The two-step conversion of various N-vinyl and N-aryl amides to the corresponding substituted pyridines and ...
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(Massachusetts Institute of Technology, 1994)
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(Massachusetts Institute of Technology, 2011)The chemical diversity found in plants has served as a major source of inspiration to many synthetic and biological chemists. Nature has evolved enzyme active sites to catalyze the synthesis of structurally complex compounds ...
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(Massachusetts Institute of Technology, 2006)Molybdenum complexes ... were used to synthesize polyene oligomeric compounds with up to 15 conjugated double bonds by reaction with aldehyde compounds in a Wittig-like fashion. The optical properties of highly nr-conjugated ...
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(Massachusetts Institute of Technology, 2007)Two distinct structural scaffolds elaborated from Schiff-base macrocycles were designed to study the proton-coupled electron transfer chemistry of 0-0 bond forming and activation chemistry. The "Hangman" architecture is ...
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(Massachusetts Institute of Technology, 1994)
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(Massachusetts Institute of Technology, 1994)
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(Massachusetts Institute of Technology, 2008)solid State NMR (SSNMR) can determine molecular as well as supermolecular structure and dynamics. The low signal intensities make many of these experiments prohibitively long. Dynamic Nuclear Polarization provides a method ...
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(Massachusetts Institute of Technology, 2007)Solid state NMR can probe structure and dynamics on length scales from the atomic to the supramolecular. However, low sensitivity limits its application in macromolecules. NMR sensitivity can be improved by dynamic nuclear ...
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(Massachusetts Institute of Technology, 1998)
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(Massachusetts Institute of Technology, 2002)In this thesis, several problems regarding dynamics and spectra in condensed phases are theoretically analyzed via analytical models. The thesis consists of four main topics. First, a theoretical description of single ...
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