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Browsing Department of Chemistry by Title
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(Massachusetts Institute of Technology, 2004)Chapter 1: Complexes obtained by electrophilic attack on a dinitrogen-derived terminal molybdenum nitride: Electronic structure analysis by solid state CP/MAS ¹⁵N NMR in combination ... Chapter 2. Carbene chemistry in the ...
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(Massachusetts Institute of Technology, 1995)
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(Massachusetts Institute of Technology, 2011)This thesis is dedicated to the application of a large-scale first-principles approach to study the electronic structure and quantum conductance of realistic nanomaterials. Three systems are studied using Landauer formalism, ...
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(Massachusetts Institute of Technology, 1994)
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(Massachusetts Institute of Technology, 2003)Chapter 1. Introduction: Electron Transfer in Biological Systems In many biological processes, including oxidative phosphorylation and photosynthesis, electron transfer reactions play vital roles. Electrons must be transported ...
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(Massachusetts Institute of Technology, 2016)A mechanistic understanding of electron transfer in solution will advance our understanding of many chemical processes, including heterogeneous redox catalysis and photochemistry-processes which are fundamental in energy ...
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(Massachusetts Institute of Technology, 2002)The role of electrostatics and packing in protein folding and molecular association was assessed in different biomolecular systems. A continuum electrostatic model was applied to long-range electrostatic effects in the ...
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(Massachusetts Institute of Technology, 1994)
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(Massachusetts Institute of Technology, 1996)
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(Massachusetts Institute of Technology, 2014)The highly-modified, bacterial sugar N,N'-diacetylbacillosamine (diNAcBac) has been implicated in the pathogenicity of certain microbes through its incorporation onto various protein virulence factors. In particular, ...
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(Massachusetts Institute of Technology, 1981)
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(Massachusetts Institute of Technology, 2011)Iminoacetonitriles participate as reactive dienophiles in intramolecular Diels-Alder cycloadditions affording quinolizidines and indolizidines. The resulting a-amino nitrile cycloadducts are versatile intermediates that ...
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(Massachusetts Institute of Technology, 2012)A method for the nickel-catalyzed cross-coupling between benzoxazole and secondary halides was explored. This method was to make use of the activated C-H bond found in benzoxazole at the 2-position to generate the nucleophilic ...
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(Massachusetts Institute of Technology, 2005)I. Enantioselective Nickel-Catalyzed Reductive Couplings of Alkynes and Aldehydes Allylic alcohol synthesis via a nickel-catalyzed reductive coupling reaction of alkylsubstituted alkynes and aldehydes was studied for ligand ...
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(Massachusetts Institute of Technology, 2007)Chapter 1 describes the development of an asymmetric nucleophile-catalyzed [2+2] cycloaddition of ketenes with aldehydes. This is the first report of a catalytic enantioselective synthesis of trisubstituted [beta]-lactones. ...
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(Massachusetts Institute of Technology, 2004)(cont.) imine.
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(Massachusetts Institute of Technology, 2010)I. Enantioselective Total Synthesis of (-)-Acylfulvene, and (-)-Irofulven We report the enantioselective total synthesis of (-)-acylfulvene and (-)-irofulven, which features metathesis reactions for the rapid assembly of ...
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(Massachusetts Institute of Technology, 2012)I. Total Synthesis of the (-)-Agelastatin Alkaloids The pyrrole-imidazole family of marine alkaloids, derived from linear clathrodin-like precursors, constitutes a diverse array of structurally complex natural products. ...
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(Massachusetts Institute of Technology, 2011)Chapter I. Introduction to the Ladder Polyethers. We introduce the bioactivity of the ladder polyether natural products and provide an overview of the puzzle that is their biogenesis. Cascades of endo-selective epoxide ...
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(Massachusetts Institute of Technology, 2009)This thesis focuses on the energetics of !-helix formation in peptides and proteins. The [alpha]-helix is the most prevalent type of secondary structure found in proteins, and has arguably dominated our thinking about ...
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