NiNC Catalysts in CO2-to-CO Electrolysis
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40820_2024_Article_1595.pdf
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Author(s) • •
Zhang, Hao
Qi, Menghui
Wang, Yong
Date Issued
December 26, 2024
Journal
Nano-Micro Letters
Publisher
Springer Nature Singapore
Citation
Zhang, H., Qi, M. & Wang, Y. NiNC Catalysts in CO2-to-CO Electrolysis. Nano-Micro Lett. 17, 94 (2025).
Version
Final published version
Abstract
CO2-to-CO electrolyzer technology converts carbon dioxide into carbon monoxide using electrochemical methods, offering significant environmental and energy benefits by aiding in greenhouse gas mitigation and promoting a carbon circular economy. Recent study by Strasser et al. in Nature Chemical Engineering presents a high-performance CO2-to-CO electrolyzer utilizing a NiNC catalyst with nearly 100% faradaic efficiency, employing innovative diagnostic tools like the carbon crossover coefficient (CCC) to address transport-related failures and optimize overall efficiency. Strasser’s research demonstrates the potential of NiNC catalysts, particularly NiNC-IMI, for efficient CO production in CO2-to-CO electrolyzers, highlighting their high selectivity and performance. However, challenges such as localized CO2 depletion and mass transport limitations underscore the need for further optimization and development of diagnostic tools like CCC. Strategies for optimizing catalyst structure and operational parameters offer avenues for enhancing the performance and reliability of electrochemical CO2 reduction catalysts.
MIT Department
Massachusetts Institute of Technology. Department of Chemical Engineering
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DOI of Published Version
https://doi.org/10.1007/s40820-024-01595-y