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Reversible high-pressure carbon nanotube vessel

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Author(s)
Wang, Lifeng
•
Ma, Ming D.
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Liu, Jefferson Z.
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Shen, Luming
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Xie, Lin
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Wei, Fei
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Zhu, Jing
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Gong, Qianming
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Liang, Ji
•
Zheng, Quanshui
Date Issued
June 2010
Journal
Physical Review B
Publisher
American Physical Society
Citation
Ma, Ming D. et al. “Reversible high-pressure carbon nanotube vessel.” Physical Review B 81.23 (2010): 235420. © 2010 The American Physical Society.
Version
Final published version
Abstract
Applying a full pressure loop, i.e., loading and unloading, on a nanocrystal with in situ observation remains a challenge to experimentalists up until now. Using a multiwalled carbon nanotube, we realize the pressure loop acting on a Fe3C nanocrystal (with peak value 20 GPa) by electron-beam irradiation with in situ observations inside transmission electron microscopy at 500 °C/ambient temperature. Using density-functional theory calculations, we attribute the unloading process to the formation of one dangling-bond single vacancies under the electron-beam irradiation at room temperature. A theoretical model is presented to understand the process and the results agree well with the experimental measurements.
MIT Department
Massachusetts Institute of Technology. Department of Mechanical Engineering
Terms of Use
Article is made available in accordance with the publisher's policy and may be subject to US copyright law. Please refer to the publisher's site for terms of use.
Persistent DSpace Link
http://hdl.handle.net/1721.1/60909
DOI of Published Version
https://doi.org/10.1103/PhysRevB.81.235420
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