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Coherent control of optical phonons in bismuth

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Author(s)
Cheng, Yu-Hsiang
•
Gao, Frank Y.
•
Teitelbaum, Samuel Welch
•
Nelson, Keith Adam
Date Issued
October 2017
Journal
Physical Review B
Publisher
American Physical Society
Citation
Cheng, Yu-Hsiang et al. “Coherent Control of Optical Phonons in Bismuth.” Physical Review B 96, 13 (October 2017): 134302 © 2017 American Physical Society
Version
Final published version
Abstract
We have conducted degenerate pump-pump-probe experiments on semimetal bismuth with femtosecond time resolution, varying both pump-probe and interpump time delays. The observed phonon dynamics, including the amplitude, damping, frequency, and phase, can be modeled by the interference of two chirped damped oscillators. No lattice anharmonicity along the trigonal axis is observed. We also find evidence of phonon-mediated relaxation of the energy density at the sample surface.
MIT Department
Massachusetts Institute of Technology. Department of Chemistry
Massachusetts Institute of Technology. Department of Electrical Engineering and Computer Science
Terms of Use
Article is made available in accordance with the publisher's policy and may be subject to US copyright law. Please refer to the publisher's site for terms of use.
Persistent DSpace Link
http://hdl.handle.net/1721.1/113382
DOI of Published Version
https://doi.org/10.1103/PhysRevB.96.134302
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