Dynamic susceptibility of supercooled water and its relation to the dynamic crossover phenomenon
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Zhang-2009-Dynamic susceptibili.pdf
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Author(s)
Zhang, Yang
Lagi, Marco
Fratini, Emiliano
Baglioni, Piero
Mamontov, Eugene
Chen, Sow-Hsin
Date Issued
April 2009
Journal
Physical Review E
Publisher
American Physical Society
Citation
Zhang, Yang et al. “Dynamic susceptibility of supercooled water and its relation to the dynamic crossover phenomenon.” Physical Review E 79.4 (2009): 040201. (C) 2010 The American Physical Society.
Version
Final published version
Abstract
We study the dynamic susceptibility χT(Q,t) of deeply supercooled water by means of quasielastic neutron scattering and molecular dynamics simulations. Both techniques show an increase in the peak height of χT(Q,t) as the temperature is lowered toward the dynamic crossover temperature TL. Below TL, the peak height decreases steadily. We attribute this phenomenon to the change in slope of the Arrhenius plot of the translational relaxation time at TL. In contrast, the peak height of the calculated four-point correlation function χ4(Q,t), directly related to the size of dynamic heterogeneity, increases toward and below TL.
MIT Department
Massachusetts Institute of Technology. Department of Nuclear Science and Engineering
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DOI of Published Version
http://dx.doi.org/10.1103/PhysRevE.79.040201
