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Initial system-environment correlations via the transfer-tensor method

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Author(s)
Buser, Maximilian
•
Cerrillo, Javier
•
Schaller, Gernot
•
Cao, Jianshu
Date Issued
December 2017
Journal
Physical Review A
Publisher
American Physical Society
Citation
Buser, Maximilian et al. "Initial system-environment correlations via the transfer-tensor method." Physical Review A 96, 6 (December 2017): 062122 © 2017 American Physical Society
Version
Final published version
Abstract
Open quantum systems exhibiting initial system-environment correlations are notoriously difficult to simulate. We point out that given a sufficiently long sample of the exact short-time evolution of the open system dynamics, one may employ transfer tensors for the further propagation of the reduced open system state. This approach is numerically advantageous and allows for the simulation of quantum correlation functions in hardly accessible regimes. We benchmark this approach against analytically exact solutions and exemplify it with the calculation of emission spectra of multichromophoric systems as well as for the reverse temperature estimation from simulated spectroscopic data. Finally, we employ our approach for the detection of spectral signatures of electromagnetically induced transparency in open three-level systems.
MIT Department
Massachusetts Institute of Technology. Department of Chemistry
Terms of Use
Article is made available in accordance with the publisher's policy and may be subject to US copyright law. Please refer to the publisher's site for terms of use.
Persistent DSpace Link
http://hdl.handle.net/1721.1/112953
DOI of Published Version
https://doi.org/10.1103/PhysRevA.96.062122
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