A Parametric Study of Multi-Stage Chemical Looping Combustion for CO[subscript 2] Capture Power Plant
Author(s)
Hassan, Bilal
Shamim, Tariq
Ghoniem, Ahmed F
Date Issued
July 2012
Journal
Proceedings of the ASME 2012 Summer Heat Transfer Conference
Publisher
ASME International
Citation
Hassan, Bilal, Tariq Shamim, and Ahmed F. Ghoniem. “A Parametric Study of Multi-Stage Chemical Looping Combustion for CO[subscript 2] Capture Power Plant.” Proceedings of the ASME 2012 Summer Heat Transfer Conference, 8-12 July, 2012, Rio Grande, Puerto Rico, ASME, 2012. © 2012 by ASME.
Version
Final published version
Abstract
A thermodynamic model and parametric analysis of a natural gas fired power plant with carbon dioxide (CO[subscript 2]) capture using multi-stage chemical looping combustion (CLC) are presented. CLC is an innovative concept and an attractive option to capture CO[subscript 2] with a significantly lower energy penalty than other carbon-capture technologies. The principal idea behind CLC is to split the combustion process into two separate steps (redox reactions) carried out in two separate reactors: an oxidation reaction and a reduction reaction, by introducing suitable metal oxide which acts as an oxygen-carrier that circulates between the two reactors. In this study, an Aspen Plus model was developed by employing the conservation of mass and energy for all the components of the CLC system. In the analysis, equilibrium based thermodynamic reactions with no oxygen-carrier deactivation were considered. The model was employed to investigate the effect of various key operating parameters such as air, fuel and oxygen carrier (OC) mass flow rates, operating pressure, and waste heat recovery on the performance of a natural gas fired power plant with multi-stage CLC. Results of these parameters on the plant efficiency are presented. The analysis shows efficiency gain of more than 6% over that of conventional power plant with CO[subscript 2] capture technologies when CLC is integrated with the power plant.
MIT Department
Massachusetts Institute of Technology. Department of Mechanical Engineering
Terms of Use
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Persistent DSpace Link
DOI of Published Version
https://doi.org/10.1115/HT2012-58597
