Screening Oxide Support Materials for OER Catalysts in Acid
Name
J. Electrochem. Soc.-2018-Han-F813-20.pdf
Description
Published version
Size
1.13 MB
Format
Adobe PDF
Checksum (MD5)
678c3ba45504ae822bc2e5a994562874
Author(s) • • • • • •
Han, Binghong
Risch, Marcel
Belden, Samuel
Lee, Seonggyu
Bayer, Domnik
Mutoro, Eva
Shao-Horn, Yang
Date Issued
July 2018
Journal
Journal of The Electrochemical Society
Publisher
The Electrochemical Society
Citation
Han, Binghong et al., "Screening Oxide Support Materials for OER Catalysts in Acid." Journal of The Electrochemical Society 165, 10 (July 2018): F813-F820 ©2018 Authors
Version
Final published version
Abstract
The lack of stable and economic supporting materials at high voltages hampers the development of electrocatalysts for oxygen evolution reaction (OER), which is the major source of energy loss in water splitting to produce hydrogen. In this work, we developed systematic methods to evaluate candidate compounds that can potentially replace traditional carbon support for OER catalysts. Stability, economic and conductivity criteria of the oxide support materials were studied and discussed. A nano-sized antimony-doped tin oxide was fabricated to support RuO2, which was shown to provide the highest stability and activity of OER in 0.5 M H2SO4 up to 2.5 VRHE and up to 55°C. ©2018 Electrochemical Society Inc.. All rights reserved.
MIT Department
Massachusetts Institute of Technology. Department of Materials Science and Engineering
Massachusetts Institute of Technology. Research Laboratory of Electronics
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DOI of Published Version
https://doi.org/10.1149/2.0921810JES