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Fundamental Limits to Extinction by Metallic Nanoparticles

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Author(s)
DeLacy, Brendan G.
•
Miller, Owen D.
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Hsu, Chia Wei
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Reid, M. T. Homer
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Soljacic, Marin
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Qiu, Wenjun
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Joannopoulos, John
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Johnson, Steven G
Date Issued
March 2014
Journal
Physical Review Letters
Publisher
American Physical Society
Citation
Miller, O. D., C. W. Hsu, M. T. H. Reid, W. Qiu, B. G. DeLacy, J. D. Joannopoulos, M. Soljacic, and S. G. Johnson. “Fundamental Limits to Extinction by Metallic Nanoparticles.” Physical Review Letters 112, no. 12 (March 2014).
Version
Final published version
Abstract
We show that there are shape-independent upper bounds to the extinction cross section per unit volume of dilute, randomly arranged nanoparticles, given only material permittivity. Underlying the limits are restrictive sum rules that constrain the distribution of quasistatic eigenvalues. Surprisingly, optimally designed spheroids, with only a single quasistatic degree of freedom, reach the upper bounds for four permittivity values. Away from these permittivities, we demonstrate computationally optimized structures that surpass spheroids and approach the fundamental limits.
MIT Department
Massachusetts Institute of Technology. Institute for Soldier Nanotechnologies
Massachusetts Institute of Technology. Department of Mathematics
Massachusetts Institute of Technology. Department of Physics
Terms of Use
Article is made available in accordance with the publisher's policy and may be subject to US copyright law. Please refer to the publisher's site for terms of use.
Persistent DSpace Link
http://hdl.handle.net/1721.1/85988
DOI of Published Version
https://doi.org/10.1103/PhysRevLett.112.123903
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