Facile and Scalable Preparation of Graphene Oxide-Based Magnetic Hybrids for Fast and Highly Efficient Removal of Organic Dyes
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Jiao-2015-Facile and scalable.pdf
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Author(s) • • • • • • • • •
Jiao, Tifeng
Liu, Yazhou
Wu, Yitian
Zhang, Qingrui
Yan, Xuehai
Gao, Faming
Bauer, Adam J. P.
Liu, Jianzhao
Zeng, Tingying
Li, Bingbing
Date Issued
July 2015
Journal
Scientific Reports
Publisher
Nature Publishing Group
Citation
Jiao, Tifeng, Yazhou Liu, Yitian Wu, Qingrui Zhang, Xuehai Yan, Faming Gao, Adam J. P. Bauer, Jianzhao Liu, Tingying Zeng, and Bingbing Li. “Facile and Scalable Preparation of Graphene Oxide-Based Magnetic Hybrids for Fast and Highly Efficient Removal of Organic Dyes.” Scientific Reports 5 (July 29, 2015): 12451.
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Final published version
Abstract
This study reports the facile preparation and the dye removal efficiency of nanohybrids composed of graphene oxide (GO) and Fe[subscript 3]O[subscript 4] nanoparticles with various geometrical structures. In comparison to previously reported GO/Fe[subscript 3]O[subscript 4] composites prepared through the one-pot, in situ deposition of Fe[subscript 3]O[subscript 4] nanoparticles, the GO/Fe[subscript 3]O[subscript 4] nanohybrids reported here were obtained by taking advantage of the physical affinities between sulfonated GO and Fe[subscript 3]O[subscript 4] nanoparticles, which allows tuning the dimensions and geometries of Fe3O4 nanoparticles in order to decrease their contact area with GO, while still maintaining the magnetic properties of the nanohybrids for easy separation and adsorbent recycling. Both the as-prepared and regenerated nanohybrids demonstrate a nearly 100% removal rate for methylene blue and an impressively high removal rate for Rhodamine B. This study provides new insights into the facile and controllable industrial scale fabrication of safe and highly efficient GO-based adsorbents for dye or other organic pollutants in a wide range of environmental-related applications.
MIT Department
Massachusetts Institute of Technology. Research Laboratory of Electronics
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DOI of Published Version
https://doi.org/10.1038/srep12451