Mass Transport and Reactions in the Tube-in-Tube Reactor
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Jensen_Tube-in-tube with SI.pdf
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1.26 MB
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Author(s) •
Yang, Lu
Jensen, Klavs F.
Date Issued
June 2013
Journal
Organic Process Research & Development
Publisher
American Chemical Society (ACS)
Citation
Yang, Lu, and Klavs F. Jensen. “Mass Transport and Reactions in the Tube-in-Tube Reactor.” Org. Process Res. Dev. 17, no. 6 (June 21, 2013): 927–933.
Version
Author's final manuscript
Abstract
The tube-in-tube reactor is a convenient method for implementing gas/liquid reactions on the microscale, in which pressurized gas permeates through a Teflon AF-2400 membrane and reacts with substrates in liquid phase. Here we present the first quantitative models for analytically and numerically computing gas and substrate concentration profiles within the tube-in-tube reactor. The model accurately predicts mass transfer performance in good agreement with experimental measurement. The scaling behavior and reaction limitations of the tube-in-tube reactor are predicted by modeling and compared with gas/liquid micro- and minireactors. The presented model yields new insights into the scalability and applicability of the tube-in-tube reactor.
MIT Department
Massachusetts Institute of Technology. Department of Chemical Engineering
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DOI of Published Version
https://doi.org/10.1021/op400085a