Ligand field design enables quantum manipulation of spins in Ni
<sup>2+</sup>
complexes
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d3sc04919a.pdf
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Published version
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Author(s)
Wojnar, Michael K
Kundu, Krishnendu
Kairalapova, Arailym
Wang, Xiaoling
Ozarowski, Andrew
Berkelbach, Timothy C
Hill, Stephen
Freedman, Danna E
Date Issued
2024
Journal
Chemical Science
Publisher
Royal Society of Chemistry (RSC)
Citation
Michael K. Wojnar, Krishnendu Kundu, Arailym Kairalapova, Xiaoling Wang, Andrew Ozarowski, Timothy C. Berkelbach, Stephen Hill, Danna E. Freedman; Ligand field design enables quantum manipulation of spins in Ni2+ complexes. Chem. Sci. 2024; 15 (4): 1374–1383.
Version
Final published version
Abstract
Molecular qubits with the potential for optical read-out require careful ligand design to control zero-field splitting, D , for quantum manipulation. We find Ni 2+ in a sulfur ligand field in a near-ideal octahedral environment enables quantum control.
Molecular qubits with the potential for optical read-out require careful ligand design to control zero-field splitting, D , for quantum manipulation. We find Ni 2+ in a sulfur ligand field in a near-ideal octahedral environment enables quantum control.
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DOI of Published Version
https://doi.org/10.1039/d3sc04919a
