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Ten-percent solar-to-fuel conversion with nonprecious materials

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Author(s)
Buonassisi, Tonio
•
Lee, Jungwoo
•
Cox, Casandra Rose
•
Nocera, Daniel G.
Date Issued
September 2014
Journal
Proceedings of the National Academy of Sciences of the United States of America
Publisher
National Academy of Sciences (U.S.)
Citation
Cox, C. R., J. Z. Lee, D. G. Nocera, and T. Buonassisi. “Ten-Percent Solar-to-Fuel Conversion with Nonprecious Materials.” Proceedings of the National Academy of Sciences 111, no. 39 (September 15, 2014): 14057–14061.
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Final published version
Abstract
Direct solar-to-fuels conversion can be achieved by coupling a photovoltaic device with water-splitting catalysts. We demonstrate that a solar-to-fuels efficiency (SFE) > 10% can be achieved with nonprecious, low-cost, and commercially ready materials. We present a systems design of a modular photovoltaic (PV)–electrochemical device comprising a crystalline silicon PV minimodule and low-cost hydrogen-evolution reaction and oxygen-evolution reaction catalysts, without power electronics. This approach allows for facile optimization en route to addressing lower-cost devices relying on crystalline silicon at high SFEs for direct solar-to-fuels conversion.
MIT Department
Massachusetts Institute of Technology. Department of Mechanical Engineering
Terms of Use
Article is made available in accordance with the publisher's policy and may be subject to US copyright law. Please refer to the publisher's site for terms of use.
Persistent DSpace Link
http://hdl.handle.net/1721.1/96320
DOI of Published Version
https://doi.org/10.1073/pnas.1414290111
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