Design of the Local Spin Polarization at the Organic-Ferromagnetic Interface
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Author(s) • • • • • •
Lazic, Predrag
Atodiresei, Nicolae
Brede, Jens
Caciuc, Vasile
Hoffmann, Germar
Wiesendanger, Roland
Blügel, Stefan
Date Issued
August 2010
Journal
Physical Review Letters
Publisher
American Physical Society
Citation
Atodiresei, Nicolae et al. “Design of the Local Spin Polarization at the Organic-Ferromagnetic Interface.” Physical Review Letters 105.6 (2010): 066601. © 2010 The American Physical Society.
Version
Final published version
Abstract
By means of ab initio calculations and spin-polarized scanning tunneling microscopy experiments the creation of a complex energy dependent magnetic structure with a tailored spin-polarized interface is demonstrated. We show this novel effect by adsorbing organic molecules containing π(pz) electrons onto a magnetic surface. The hybridization of the out-of-plane pz atomic-type orbitals with the d states of the metal leads to the inversion of the spin polarization at the organic site due to a pz-d Zener exchange-type mechanism. As a key result, we demonstrate the possibility to selectively and efficiently inject spin-up and spin-down electrons from a ferromagnetic-organic interface, an effect which can be exploited in future spintronic devices.
MIT Department
Massachusetts Institute of Technology. Department of Materials Science and Engineering
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DOI of Published Version
https://doi.org/10.1103/PhysRevLett.105.066601