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Stratospheric Ozone in the Last Glacial Maximum
Name
2020JD032929.pdf
Description
Published version
Size
6.3 MB
Format
Adobe PDF
Checksum (MD5)
202ee6c3ac8792a71e90a81870552828
Author(s)
Wang, Mingcheng
Fu, Qiang
Solomon, Susan
White, Rachel H
Alexander, Becky
Date Issued
2020
Journal
Journal of Geophysical Research: Atmospheres
Publisher
American Geophysical Union (AGU)
Version
Final published version
Abstract
©2020. The Authors. Using the Whole Atmosphere Community Climate Model version 6, stratospheric ozone in the Last Glacial Maximum (LGM) is investigated. It is shown that, compared with preindustrial (PI) times, LGM modeled stratospheric temperatures are increased by up to 8 K, leading to faster ozone destruction rates for gas phase reactions, especially via the Chapman mechanism. On the other hand, stratospheric hydroxyl radical (OH) and nitrogen oxides (NOx) concentrations are decreased by 10–20%, which decreases catalytic ozone destruction, thereby decreasing ozone loss rates. The net effect of these two compensating mechanisms in the upper stratosphere (above 15 hPa) is a vertically integrated 1–3 Dobson unit (DU) decrease during the LGM. In the lower stratosphere (tropopause to 15 hPa), changes in the stratospheric overturning circulation and resulting transport dominate changes in ozone. Consistent with a weakening of the residual circulation in the LGM, lower stratospheric ozone is increased by 2–5 DU in the tropics and decreased by 5–10 DU in the extratropics, but the latter is partly compensated by ozone increases due to a lower tropopause. It is found that tropospheric ozone is decreased by about 5 DU in the LGM versus PI. Combined changes in stratospheric and tropospheric ozone lead to a decrease in total ozone column everywhere except over the northeast North America, equatorial Indian and West Pacific Oceans. Surface ultraviolet radiation in the LGM versus PI is increased over the Northern Hemisphere middle and high latitudes, especially over the ice caps, and over the Southern Hemisphere near 60°S.
Terms of Use
Creative Commons Attribution 4.0 International license
Persistent DSpace Link
DOI of Published Version
10.1029/2020JD032929
