Photo-excitation Cascade and Multiple Carrier Generation in Graphene
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Levitov_Photoexcitation.pdf
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Author(s)
Tielrooij, K. J.
Jensen, S. A.
Centeno, A.
Pesquera, A.
Zurutuza Elorza, A.
Bonn, M.
Koppens, Frank Henricus Louis
Song, Justin Chien Wen
Levitov, Leonid
Alternative Title
Photoexcitation cascade and multiple hot-carrier generation in graphene
Date Issued
February 2013
Journal
Nature Physics
Publisher
Nature Publishing Group
Citation
Tielrooij, K. J., J. C. W. Song, S. A. Jensen, A. Centeno, A. Pesquera, A. Zurutuza Elorza, M. Bonn, L. S. Levitov, and F. H. L. Koppens. “Photoexcitation Cascade and Multiple Hot-Carrier Generation in Graphene.” Nat Phys 9, no. 4 (February 24, 2013): 248–252.
Version
Author's final manuscript
Abstract
The conversion of light into free electron–hole pairs constitutes the key process in the fields of photodetection and photovoltaics. The efficiency of this process depends on the competition of different relaxation pathways and can be greatly enhanced when photoexcited carriers do not lose energy as heat, but instead transfer their excess energy into the production of additional electron–hole pairs through carrier–carrier scattering processes. Here we use optical pump–terahertz probe measurements to probe different pathways contributing to the ultrafast energy relaxation of photoexcited carriers. Our results indicate that carrier–carrier scattering is highly efficient, prevailing over optical-phonon emission in a wide range of photon wavelengths and leading to the production of secondary hot electrons originating from the conduction band. As hot electrons in graphene can drive currents, multiple hot-carrier generation makes graphene a promising material for highly efficient broadband extraction of light energy into electronic degrees of freedom, enabling high-efficiency optoelectronic applications.
MIT Department
Massachusetts Institute of Technology. Department of Physics
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DOI of Published Version
https://doi.org/10.1038/nphys2564
