Tunable and Responsive Structural Color from Polymeric Microstructured Surfaces Enabled by Interference of Totally Internally Reflected Light
Name
ACS Materials Letters - with figures embedded.pdf
Description
Accepted version
Size
1.52 MB
Format
Adobe PDF
Checksum (MD5)
6ee7b4a1be7d9fd9a5e9f20a20faf1b3
Author(s)
Goodling, Amy E.
Nagelberg, Sara
Kolle, Mathias
Zarzar, Lauren D.
Date Issued
May 27, 2020
Journal
ACS Materials Letters
Publisher
American Chemical Society
Citation
ACS Materials Lett. 2020, 2, 7, 754–763.
Version
Author's final manuscript
Abstract
This report describes a straightforward and versatile approach to the fabrication of polymer films composed of microscale dome or well features that create structural color by interference from total internal reflection. The fabrication approach utilizes assembly of glass particles at monomer oil-water interfaces, providing control over the radius of curvature and contact angle of the resultant microstructures. The influence of the microscale concave interface geometry and refractive index contrast on the structural colors produced is systematically investigated, and the results are compared with those predicted by optical modeling. By dynamically changing such parameters, for example, by deforming the surfaces with mechanical force or using temperature to change refractive index, stimuli-responsive color-changing surfaces and structurally colored patterned images are demonstrated. This simple design and fabrication method to produce structurally colored surfaces may be of interest for both fundamental and applied research areas such as dynamic displays, anticounterfeiting technology, and colorimetric sensors.
MIT Department
Massachusetts Institute of Technology. Department of Mechanical Engineering
Terms of Use
Creative Commons Attribution-Noncommercial-ShareAlike
Persistent DSpace Link
DOI of Published Version
https://doi.org/10.1021/acsmaterialslett.0c00143
