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Synthesis, characterization, and biotemplated assembly of indium nitride and indium gallium nitride nanoparticles

Author(s)
Hsieh, Jennifer Chia-Jen
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Massachusetts Institute of Technology. Dept. of Materials Science and Engineering.
Advisor
Angela M. Belcher.
Terms of use
M.I.T. theses are protected by copyright. They may be viewed from this source for any purpose, but reproduction or distribution in any format is prohibited without written permission. See provided URL for inquiries about permission. http://dspace.mit.edu/handle/1721.1/7582
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Abstract
A low-temperature, ambient pressure solution synthesis of colloidal InN nanoparticles is presented. This synthesis utilizes a previously dismissed precursor and results in individual, non-aggregated nanoparticles with long-term solubility and stability in organic solvents. These nanoparticles are wurtzite phase with a measured bandgap as low as 0.79 eV and average size of 6.2 nm. Based on this synthesis, indium-rich InGaN nanoparticles were synthesized and characterized. Chemical, structural, and optical analysis indicated up to 10% gallium incorporation before encountering the miscibility gap. Using CdSe nanoparticles as a model system, M13 bacteriophage-mediated, two-dimensional nanoparticle assembly was examined as a route for scaleable, large-area nanoparticle films. The method uses close-packed, self-assembly of M13 on layer-by-layer deposited polyelectrolyte surfaces and was able to assemble aminated nanoparticles with strong specificity.
Description
Thesis (Ph. D.)--Massachusetts Institute of Technology, Dept. of Materials Science and Engineering, 2010.
 
Cataloged from PDF version of thesis.
 
Includes bibliographical references.
 
Date issued
2010
URI
http://hdl.handle.net/1721.1/59706
Department
Massachusetts Institute of Technology. Department of Materials Science and Engineering
Publisher
Massachusetts Institute of Technology
Keywords
Materials Science and Engineering.

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