Lead-related quantum emitters in diamond
Name
PhysRevB.99.075430.pdf
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Author(s) • • • • • • • • •
Ciccarino, Christopher J.
Flick, Johannes
Sundararaman, Ravishankar
Malladi, Girish
Walsh, Michael
Bakhru, Hassaram
Narang, Prineha
Trusheim, Matthew E
Wan, Noel Heng Loon
Chen, Kevin C.
Date Issued
February 2019
Journal
Physical Review B
Publisher
American Physical Society
Citation
Trusheim, Matthew E., et al. “Lead-Related Quantum Emitters in Diamond.” Physical Review B, vol. 99, no. 7, Feb. 2019. © 2019 American Physical Society
Version
Final published version
Abstract
We report on quantum emission from Pb-related color centers in diamond following ion implantation and high-temperature vacuum annealing. First-principles calculations predict a negatively charged Pb-vacancy (PbV) center in a split-vacancy configuration, with a zero-phonon transition around 2.4 eV. Cryogenic photoluminescence measurements performed on emitters in nanofabricated pillars reveal several transitions, including a prominent doublet near 520 nm. The splitting of this doublet, 5.7 THz, exceeds that reported for other group-IV centers. These observations are consistent with the PbV center, which is expected to have a combination of narrow optical transitions and stable spin states, making it a promising system for quantum network nodes.
MIT Department
Massachusetts Institute of Technology. Department of Electrical Engineering and Computer Science
Massachusetts Institute of Technology. Research Laboratory of Electronics
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DOI of Published Version
https://doi.org/10.1103/PhysRevB.99.075430