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Lead-related quantum emitters in diamond

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PhysRevB.99.075430.pdf

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Author(s)
Ciccarino, Christopher J.
•
Flick, Johannes
•
Sundararaman, Ravishankar
•
Malladi, Girish
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Walsh, Michael
•
Bakhru, Hassaram
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Narang, Prineha
•
Trusheim, Matthew E
•
Wan, Noel Heng Loon
•
Chen, Kevin C.
more
Date Issued
February 2019
Journal
Physical Review B
Publisher
American Physical Society
Citation
Trusheim, Matthew E., et al. “Lead-Related Quantum Emitters in Diamond.” Physical Review B, vol. 99, no. 7, Feb. 2019. © 2019 American Physical Society
Version
Final published version
Abstract
We report on quantum emission from Pb-related color centers in diamond following ion implantation and high-temperature vacuum annealing. First-principles calculations predict a negatively charged Pb-vacancy (PbV) center in a split-vacancy configuration, with a zero-phonon transition around 2.4 eV. Cryogenic photoluminescence measurements performed on emitters in nanofabricated pillars reveal several transitions, including a prominent doublet near 520 nm. The splitting of this doublet, 5.7 THz, exceeds that reported for other group-IV centers. These observations are consistent with the PbV center, which is expected to have a combination of narrow optical transitions and stable spin states, making it a promising system for quantum network nodes.
MIT Department
Massachusetts Institute of Technology. Department of Electrical Engineering and Computer Science
Massachusetts Institute of Technology. Research Laboratory of Electronics
Terms of Use
Article is made available in accordance with the publisher's policy and may be subject to US copyright law. Please refer to the publisher's site for terms of use.
Persistent DSpace Link
http://hdl.handle.net/1721.1/121092
DOI of Published Version
https://doi.org/10.1103/PhysRevB.99.075430
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