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dc.contributor.authorWu, Albert
dc.contributor.authorDrayton, James A.
dc.contributor.authorSmith, Zachary P
dc.date.accessioned2020-02-21T20:09:12Z
dc.date.available2020-02-21T20:09:12Z
dc.date.issued2019-06
dc.date.submitted2019-03
dc.identifier.issn0001-1541
dc.identifier.issn1547-5905
dc.identifier.urihttps://hdl.handle.net/1721.1/123841
dc.description.abstractPerfluoropolymers have fundamentally distinct thermodynamic partitioning properties compared to those of their hydrocarbon counterparts. However, current upper bound theory assumes hydrocarbon solubility behavior for all polymers. Herein, the fundamental presupposition of invariance in solubility behavior to upper bound performance is critically assessed for perfluoropolymers and hydrocarbon polymers. By modifying solubility relationships, theoretical perfluoropolymer upper bounds are established, showing a positive shift of the upper bound front as a result of beneficial solubility selectivities for certain gas pairs, including N₂/CH₄, He/H₂, He/N₂, He/CH₄, and He/CO₂. Within the framework of the solution–diffusion model, an analysis is presented to compare two independent approaches often pursued in efforts to surpass the polymer upper bound: (a) achieving solubility selectivity via perfluoropolymers and (b) improving diffusion selectivity via rigid hydrocarbon polymers. This analysis demonstrates the significant benefit that can be achieved by considering both the chemical composition and morphology of solid‐state macromolecules when designing membrane materials. Keywords: activated diffusion theory; membrane‐based separations; perfluorocarbon; solubilityen_US
dc.description.sponsorshipNational Science Foundation (U.S.) (Grant 1122374)en_US
dc.description.sponsorshipAmerican Chemical Society (Grant 59256‐DNI7)
dc.publisherWileyen_US
dc.relation.isversionofhttp://dx.doi.org/10.1002/aic.16700en_US
dc.rightsCreative Commons Attribution-Noncommercial-Share Alikeen_US
dc.rights.urihttp://creativecommons.org/licenses/by-nc-sa/4.0/en_US
dc.sourceProf. Zachary Smithen_US
dc.titleThe perfluoropolymer upper bounden_US
dc.typeArticleen_US
dc.identifier.citationWu, Albert X. et al. "The perfluoropolymer upper bound." AIChE Journal 65, 12 (June 2019): e16700 © 2019 American Institute of Chemical Engineers
dc.contributor.departmentMassachusetts Institute of Technology. Department of Chemical Engineeringen_US
dc.relation.journalAIChE Journalen_US
dc.eprint.versionAuthor's final manuscripten_US
dc.type.urihttp://purl.org/eprint/type/JournalArticleen_US
eprint.statushttp://purl.org/eprint/status/PeerRevieweden_US
dc.identifier.doi10.1002/aic.16700en_US
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dspace.date.submission2020-02-13T15:19:12Z
mit.journal.volume65en_US
mit.journal.issue12en_US
mit.licenseOPEN_ACCESS_POLICY
mit.metadata.statusComplete


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