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dc.contributor.authorHaji, Maha N.
dc.contributor.authorDrysdale, Jessica A.
dc.contributor.authorHaji, Maha Niametullah
dc.contributor.authorBuesseler, Ken O.
dc.contributor.authorSlocum, Alexander H.
dc.date.accessioned2020-10-08T22:54:02Z
dc.date.available2020-10-08T22:54:02Z
dc.date.issued2019-01-16
dc.date.submitted2018-12
dc.identifier.issn0013-936X
dc.identifier.issn1520-5851
dc.identifier.urihttps://hdl.handle.net/1721.1/127940
dc.description.abstractAmidoxime-based adsorbents have become highly promising for seawater uranium extraction. However, current deployment schemes are stand-alone, intermittent operation systems that have significant practical and economic challenges. This paper presents two 1:10 scale prototypes of a Symbiotic Machine for Ocean uRanium Extraction (SMORE) which pairs with an existing offshore structure. This pairing reduces mooring and deployment costs while enabling continuous, autonomous uranium extraction. Utilizing a shell enclosure to decouple the mechanical and chemical requirements of the adsorbent, one design concept prototyped continuously moves the shells through the water while the other keeps them stationary. Water flow in the shells on each prototype was determined using the measurement of radium adsorbed by MnO 2 impregnated acrylic fibers contained within each enclosure. The results from a nine-week ocean trial show that while movement of the shells through the water may not have an effect on uranium adsorption by the fibers encased, it could help reduce biofouling if above a certain threshold speed (resulting in increased uptake), while also allowing for the incorporation of design elements to further mitigate biofouling such as bristle brushes and UV lamps. The trace metal uptake by the AI8 adsorbents in this trial also varied greatly from previous marine deployments, suggesting that uranium uptake may depend greatly upon the seawater concentrations of other elements such as vanadium and copper. The results from this study will be used to inform future work on the seawater uranium production cost from a full-scale SMORE system.en_US
dc.description.sponsorshipU.S. Department of Energy Office of Nuclear Energy (Contracts DE-NE0008268 and DE-NE000731)en_US
dc.language.isoen
dc.publisherAmerican Chemical Society (ACS)en_US
dc.relation.isversionofhttp://dx.doi.org/10.1021/acs.est.8b05100en_US
dc.rightsArticle is made available in accordance with the publisher's policy and may be subject to US copyright law. Please refer to the publisher's site for terms of use.en_US
dc.sourceProf. Slocum via Elizabeth Soergelen_US
dc.titleResults of an Ocean Trial of the Symbiotic Machine for Ocean Uranium Extractionen_US
dc.typeArticleen_US
dc.identifier.citationHaji, Maha N. et al. "Results of an Ocean Trial of the Symbiotic Machine for Ocean Uranium Extraction." Environmental Science and Technology 53, 4 (January 2019): 2229–2237 © 2019 American Chemical Societyen_US
dc.contributor.departmentMassachusetts Institute of Technology. Department of Mechanical Engineeringen_US
dc.relation.journalEnvironmental Science and Technologyen_US
dc.eprint.versionAuthor's final manuscripten_US
dc.type.urihttp://purl.org/eprint/type/JournalArticleen_US
eprint.statushttp://purl.org/eprint/status/PeerRevieweden_US
dc.date.updated2020-09-23T13:16:56Z
dspace.orderedauthorsHaji, MN; Drysdale, JA; Buesseler, KO; Slocum, AHen_US
dspace.date.submission2020-09-23T13:17:01Z
mit.journal.volume53en_US
mit.journal.issue4en_US
mit.licensePUBLISHER_POLICY
mit.metadata.statusComplete


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