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Toward New 2D Zirconium-Based Metal–Organic Frameworks: Synthesis, Structures, and Electronic Properties

Author(s)
Cadiau, Amandine; Xie, Lilia S.; Kolobov, Nikita; Shkurenko, Aleksander; Qureshi, Muhammad; Tchalala, Mohamed R.; Park, Sarah Sunah; Bavykina, Anastasiya; Eddaoudi, Mohamed; Dinca, Mircea; Hendon, Christopher H.; Gascon, Jorge; ... Show more Show less
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Abstract
Nowadays, zirconium metal-organic frameworks attract more attention because of their robustness and their easier predictability in terms of topology. Herein, we have been able to control synthetic parameters in order to construct two new 2D MOFs with the same sql topology. Both materials, ACM-10 and ACM-11, have been characterized by single-crystal X-ray diffraction, thermogravimetric analysis, and UV-vis spectroscopy. Their textural, electrochemical, and conductivity properties are presented along with the opportunities that these new topologically interesting scaffolds offer for the design of new structures.
Date issued
2019-12
URI
https://hdl.handle.net/1721.1/128213
Department
Massachusetts Institute of Technology. Department of Chemistry
Journal
Chemistry of Materials
Publisher
American Chemical Society (ACS)
Citation
Cadiau, Amandine et al. "Toward New 2D Zirconium-Based Metal–Organic Frameworks: Synthesis, Structures, and Electronic Properties." Chemistry of Materials 32, 1 (December 2019): 97–104 © 2019 American Chemical Society
Version: Author's final manuscript
ISSN
0897-4756
1520-5002

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