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Universality of electron mobility in LaAlO 3 /SrTiO 3 and bulk SrTiO 3

Author(s)
Trier, Felix; Reich, KV; Christensen, Dennis Valbjørn; Zhang, Yu; Tuller, Harry L; Chen, Yunzhong; Shklovskii, BI; Pryds, Nini; ... Show more Show less
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Abstract
© 2017 Author(s). Metallic LaAlO3/SrTiO3 (LAO/STO) interfaces attract enormous attention, but the relationship between the electron mobility and the sheet electron density, ns, is poorly understood. Here, we derive a simple expression for the three-dimensional electron density near the interface, n3D, as a function of ns and find that the mobility for LAO/STO-based interfaces depends on n3D in the same way as it does for bulk doped STO. It is known that undoped bulk STO is strongly compensated with N5×1018 cm-3 background donors and acceptors. In intentionally doped bulk STO with a concentration of electrons n3D<N, background impurities determine the electron scattering. Thus, when n3D<N, it is natural to see in LAO/STO the same mobility as in the bulk. On the other hand, in the bulk samples with n3D>N, the mobility collapses because scattering happens on n3D intentionally introduced donors. For LAO/STO, the polar catastrophe which provides electrons is not supposed to provide an equal number of random donors and thus the mobility should be larger. The fact that the mobility is still the same implies that for the LAO/STO, the polar catastrophe model should be revisited.
Date issued
2017
URI
https://hdl.handle.net/1721.1/134837
Department
Massachusetts Institute of Technology. Department of Materials Science and Engineering
Journal
Applied Physics Letters
Publisher
AIP Publishing

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