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dc.contributor.authorSaló-Salgado, Lluís
dc.contributor.authorHaugen, Malin
dc.contributor.authorEikehaug, Kristoffer
dc.contributor.authorFernø, Martin
dc.contributor.authorNordbotten, Jan M.
dc.contributor.authorJuanes, Ruben
dc.date.accessioned2024-04-19T15:22:15Z
dc.date.available2024-04-19T15:22:15Z
dc.date.issued2023-06-23
dc.identifier.issn0169-3913
dc.identifier.issn1573-1634
dc.identifier.urihttps://hdl.handle.net/1721.1/154227
dc.description.abstractThe accuracy and robustness of numerical models of geologic CO2 sequestration are almost never quantified with respect to direct observations that provide a ground truth. Here, we conduct CO2 injection experiments in meter-scale, quasi-2D tanks with porous media representing stratigraphic sections of the subsurface, and compare them to numerical simulations of those experiments. We evaluate (1) the value of prior knowledge of the system, expressed in terms of ex situ measurements of the tank sands’ multiphase flow properties (local data), with respect to simulation accuracy; and (2) the forecasting capability of history-matched numerical models, when applied to different settings. We match three versions of a numerical simulation model—each with access to an increasing level of local data—to a CO2 injection experiment in Tank 1 (89.7×47×1.05 cm). Matching is based on a quantitative comparison of CO2 migration at different times from timelapse image analysis. Next, use the matched models to make a forecast of a different injection scenario in Tank 1 and, finally, a different injection scenario in Tank 2 (2.86×1.3×0.019 m), which represents an altogether different stratigraphic section. The simulation model can qualitatively match the observed free-phase and dissolved CO2 plume migration and convective mixing. Quantitatively, simulations are accurate during the injection phase, but their concordance decreases with time. Using local data reduces the time required to history match, although the forecasting capability of matched models is similar. The sand–water–CO2(g) system is very sensitive to effective permeability and capillary pressure changes; where heterogeneous structures are present, accurate deterministic estimates of CO2 migration are difficult to obtain.en_US
dc.publisherSpringer Science and Business Media LLCen_US
dc.relation.isversionof10.1007/s11242-023-01972-yen_US
dc.rightsArticle is made available in accordance with the publisher's policy and may be subject to US copyright law. Please refer to the publisher's site for terms of use.en_US
dc.sourceSpringer Netherlandsen_US
dc.subjectGeneral Chemical Engineeringen_US
dc.subjectCatalysisen_US
dc.titleDirect Comparison of Numerical Simulations and Experiments of $$\hbox {CO}_2$$ Injection and Migration in Geologic Media: Value of Local Data and Forecasting Capabilityen_US
dc.typeArticleen_US
dc.identifier.citationSaló-Salgado, L., Haugen, M., Eikehaug, K. et al. Direct Comparison of Numerical Simulations and Experiments of CO2 Injection and Migration in Geologic Media: Value of Local Data and Forecasting Capability. Transp Porous Med 151, 1199–1240 (2024).en_US
dc.contributor.departmentMassachusetts Institute of Technology. Department of Civil and Environmental Engineering
dc.contributor.departmentMassachusetts Institute of Technology. Department of Earth, Atmospheric, and Planetary Sciences
dc.contributor.departmentMassachusetts Institute of Technology. Earth Resources Laboratory
dc.eprint.versionAuthor's final manuscripten_US
dc.type.urihttp://purl.org/eprint/type/JournalArticleen_US
eprint.statushttp://purl.org/eprint/status/PeerRevieweden_US
dc.date.updated2024-04-19T03:28:28Z
dc.language.rfc3066en
dc.rights.holderThe Author(s), under exclusive licence to Springer Nature B.V.
dspace.embargo.termsY
dspace.date.submission2024-04-19T03:28:27Z
mit.journal.volume151en_US
mit.journal.issue5en_US
mit.licensePUBLISHER_POLICY
mit.metadata.statusAuthority Work and Publication Information Neededen_US


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