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Synthesis of Photoresponsive Dual NIR Two-Photon Absorptive [60]Fullerene Triads and Tetrads

Author(s)
Jeon, Seaho; Wang, Min; Tan, Loon-Seng; Cooper, Thomas; Hamblin, Michael R.; Chiang, Long Y.; ... Show more Show less
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Abstract
Broadband nonlinear optical (NLO) organic nanostructures exhibiting both ultrafast photoresponse and a large cross-section of two-photon absorption throughout a wide NIR spectrum may make them suitable for use as nonlinear biophotonic materials. We report here the synthesis and characterization of two C60-(antenna)x analogous compounds as branched triad C60(>DPAF-C18)(>CPAF-C2M) and tetrad C60(>DPAF-C18)(>CPAF-C2M)2 nanostructures. These compounds showed approximately equal extinction coefficients of optical absorption over 400–550 nm that corresponds to near-IR two-photon based excitation wavelengths at 780–1,100 nm. Accordingly, they may be utilized as potential precursor candidates to the active-core structures of photosensitizing nanodrugs for 2γ-PDT in the biological optical window of 800–1,050 nm.
Date issued
2013-08
URI
http://hdl.handle.net/1721.1/88097
Department
Harvard University--MIT Division of Health Sciences and Technology
Journal
Molecules
Publisher
MDPI AG
Citation
Jeon, Seaho, Min Wang, Loon-Seng Tan, Thomas Cooper, Michael Hamblin, and Long Chiang. “Synthesis of Photoresponsive Dual NIR Two-Photon Absorptive [60]Fullerene Triads and Tetrads.” Molecules 18, no. 8 (August 12, 2013): 9603–9622.
Version: Final published version
ISSN
1420-3049

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