| dc.contributor.author | Bertrand, Christopher E. | |
| dc.contributor.author | Liu, K.-H. | |
| dc.contributor.author | Mamontov, Eugene | |
| dc.contributor.author | Chen, Sow-Hsin | |
| dc.date.accessioned | 2014-08-25T18:37:32Z | |
| dc.date.available | 2014-08-25T18:37:32Z | |
| dc.date.issued | 2013-04 | |
| dc.date.submitted | 2013-03 | |
| dc.identifier.issn | 1539-3755 | |
| dc.identifier.issn | 1550-2376 | |
| dc.identifier.uri | http://hdl.handle.net/1721.1/89038 | |
| dc.description.abstract | We have measured the hydration-level dependence of the single-particle dynamics of water confined in the ordered mesoporous silica MCM-41. The dynamic crossover observed at full hydration is absent at monolayer hydration. The monolayer dynamics are significantly slower than those of water in a fully hydrated pore at ambient temperatures. At low temperatures, the opposite is found to be true. These results underscore the importance of water's tetrahedral hydrogen-bond network in accounting for its low temperature dynamic properties. | en_US |
| dc.description.sponsorship | United States. Dept. of Energy. Office of Basic Energy Sciences (Contract DE-FG02-90ER45429) | en_US |
| dc.language.iso | en_US | |
| dc.publisher | American Physical Society | en_US |
| dc.relation.isversionof | http://dx.doi.org/10.1103/PhysRevE.87.042312 | en_US |
| dc.rights | Article is made available in accordance with the publisher's policy and may be subject to US copyright law. Please refer to the publisher's site for terms of use. | en_US |
| dc.source | American Physical Society | en_US |
| dc.title | Hydration-dependent dynamics of deeply cooled water under strong confinement | en_US |
| dc.type | Article | en_US |
| dc.identifier.citation | Bertrand, C. E., K.-H. Liu, E. Mamontov, and S.-H. Chen. “Hydration-Dependent Dynamics of Deeply Cooled Water Under Strong Confinement.” Phys. Rev. E 87, no. 4 (April 2013). © 2013 American Physical Society | en_US |
| dc.contributor.department | Massachusetts Institute of Technology. Department of Nuclear Science and Engineering | en_US |
| dc.contributor.mitauthor | Chen, Sow-Hsin | en_US |
| dc.contributor.mitauthor | Bertrand, Christopher E. | en_US |
| dc.contributor.mitauthor | Liu, K.-H. | en_US |
| dc.relation.journal | Physical Review E | en_US |
| dc.eprint.version | Final published version | en_US |
| dc.type.uri | http://purl.org/eprint/type/JournalArticle | en_US |
| eprint.status | http://purl.org/eprint/status/PeerReviewed | en_US |
| dspace.orderedauthors | Bertrand, C. E.; Liu, K.-H.; Mamontov, E.; Chen, S.-H. | en_US |
| dc.identifier.orcid | https://orcid.org/0000-0001-6588-2428 | |
| dspace.mitauthor.error | true | |
| mit.license | PUBLISHER_POLICY | en_US |
| mit.metadata.status | Complete | |
